A left-wing journalist I know on Bluesky was saying that the push around Greenland is clearly related to the VC-backed Network State idea. 

I spent some time yesterday perusing this website: https://www.vcinfodocs.com/what-is-the-network-state

Obviously there’s a big crypto connection. What do you guys think of the project? Anyone involved? What does this clearly very skeptical site miss?

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I think this is unlikely. At the end of the day the Network State movement does want to create communities and have people move to the sovereign states they set up. Greenland while resource rich is super inhospitable. I could more easily foresee a deal where a network state gets the ruins of Gaza than Greenland